Crystallization Process as a Final Part of Zero Liquid Discharge System for Treatment of East Baghdad Oilfield Produced Water

Authors

  • Miqat Hasan Salih Chemical Engineering Department, College of Engineering, University of Baghdad, Baghdad, Iraq
  • Ahmed Faiq Al-Alawy Chemical Engineering Department, College of Engineering, University of Baghdad, Baghdad, Iraq

DOI:

https://doi.org/10.31699/IJCPE.2022.1.3

Keywords:

Crystallization, evaporation, zero liquid discharge system, Iraqi oilfield produced water

Abstract

This study investigated the application of the crystallization process for oilfield produced water from the East Baghdad oilfield affiliated to the Midland Oil Company (Iraq). Zero liquid discharge system (ZLD) consists of several parts such as oil skimming, coagulation/flocculation, forward osmosis, and crystallization, the crystallization process is a final part of a zero liquid discharge system. The laboratory-scale simple evaporation system was used to evaluate the performance of the crystallization process. In this work, sodium chloride solution and East Baghdad oilfield produced water were used as a feed solution with a concentration of 177 and 220 g/l. The impact of temperature (70, 80, and 90 °C), mixing speed (300, 400, and 500 rpm), feed concentration (177 and 220 g/l), and time (0.5-9.5 h) on the crystallization performance for oilfield produced water treatment were investigated on evaporation rate and recovery. The recovery increased with increasing temperature and mixing speed while decreasing with an increase in feed concentration. Pure water and salts were recovered from the concentrated produced water, the recovery of pure water at 80 °C, 400 rpm, and 220 g/l feed concentration was 82.22 and 81.35% after 5.5 h for NaCl solution (i.e., simulated oilfield produced water) and oilfield produced water, respectively.

References

A. F. Al-Alawy and M. H. Salih, “Experimental Study and Mathematical Modelling of Zinc Removal by Reverse Osmosis Membranes,” Iraqi J. Chem. Pet. Eng., vol. 17, no. 3, pp. 57–73, 2016. https://doi.org/10.31699/IJCPE.2016.3.5

K. J. Lu, Z. L. Cheng, J. Chang, L. Luo, and T. S. Chung, “Design of zero liquid discharge desalination (ZLDD) systems consisting of freeze desalination, membrane distillation, and crystallization powered by green energies,” Desalination, vol. 458, pp. 66–75, 2019, doi: 10.1016/j.desal.2019.02.001.

T. Tong and M. Elimelech, “The Global Rise of Zero Liquid Discharge for Wastewater Management: Drivers, Technologies, and Future Directions,” Environ. Sci. Technol., vol. 50, no. 13, pp. 6846–6855, 2016, doi: 10.1021/acs.est.6b01000.

A. F. Al-Alawy, T. R. Abbas, and H. K. Mohammed, “Osmostic Membrane Bioreactor for Oily Wastewater Treatment using External & Internal Configurations,” Iraqi J. Chem. Pet. Eng., vol. 17, no. 4, pp. 71–82, 2016.

M. S. Al-Rubaie, M. A. Dixon, and T. R. Abbas, “Use of flocculated magnetic separation technology to treat Iraqi oilfield co-produced water for injection purpose,” Desalin. Water Treat., vol. 53, no. 8, pp. 2086–2091, 2015, doi: 10.1080/19443994.2013.860400.

B. I. H. Waisi, U. F. A. Karim, D. C. M. Augustijn, M. H. O. Al-Furaiji, and S. J. M. H. Hulscher, “A study on the quantities and potential use of produced water in southern Iraq,” Water Sci. Technol. Water Supply, vol. 15, no. 2, pp. 370–376, 2015, doi: 10.2166/ws.2014.122.

J. Zhai et al., “Comparison of coagulation pretreatment of produced water from natural gas well by polyaluminium chloride and polyferric sulphate coagulants,” Environ. Technol., vol. 38, no. 10, pp. 1200–1210, 2017, doi: 10.1080/09593330.2016.1217937.

A. A. Al-Haleem, H. H.Abdulah, and E. A.-J. Saeed, “Components and Treatments of Oilfield Produced Water,” Al-Khawarizmi Eng. J., vol. 6, no. 1, pp. 24–30, 2010.

A. A. A.-H. A.Al-Razaq, “Oilfield Produced Water Management: Treatment, Reuse and Disposal,” Baghdad Sci. J., vol. 9, no. 1, pp. 124–132, 2012, doi: 10.21123/bsj.9.1.124-132.

F. I. El-Hosiny, K. A. Selim, M. A. A. Khalek, and I. Osama, “Produced Water Treatment Using a New Designed Electroflotation Cell,” Int. J. Res. Ind. Eng., vol. 6, no. 4, pp. 328–338, 2017, doi: 10.22105/riej.2017.100959.1022.

A. Fakhru’l-Razi, A. Pendashteh, Z. Z. Abidin, L. C. Abdullah, D. R. A. Biak, and S. S. Madaeni, “Application of membrane-coupled sequencing batch reactor for oilfield produced water recycle and beneficial re-use,” Bioresour. Technol., vol. 101, no. 18, pp. 6942–6949, 2010, doi: 10.1016/j.biortech.2010.04.005.

A. Davarpanah, “Feasible analysis of reusing flowback produced water in the operational performances of oil reservoirs,” Environ. Sci. Pollut. Res., vol. 25, no. 35, pp. 35387–35395, 2018, doi: 10.1007/s11356-018-3506-9.

Y. Oren et al., “Pilot studies on high recovery BWRO-EDR for near zero liquid discharge approach,” Desalination, vol. 261, no. 3, pp. 321–330, 2010, doi: 10.1016/j.desal.2010.06.010.

Y. Shi et al., “Solar Evaporator with Controlled Salt Precipitation for Zero Liquid Discharge Desalination,” Environ. Sci. Technol., vol. 52, pp. 11822–11830, 2018, doi: 10.1021/acs.est.8b03300.

J. Grönwall and A. C. Jonsson, “The impact of ‘zero’ coming into fashion: Zero liquid discharge uptake and socio-technical transitions in Tirupur,” Water Altern., vol. 10, no. 2, pp. 602–624, 2017.

G. U. Semblante, J. Z. Lee, L. Y. Lee, S. L. Ong, and H. Y. Ng, “Brine pre-treatment technologies for zero liquid discharge systems,” Desalination, vol. 441, pp. 96–111, 2018, doi: 10.1016/j.desal.2018.04.006.

C. Finnerty, L. Zhang, D. L. Sedlak, K. L. Nelson, and B. Mi, “Synthetic Graphene Oxide Leaf for Solar Desalination with Zero Liquid Discharge,” Environ. Sci. Technol., vol. 51, no. 20, pp. 11701–11709, 2017, doi: 10.1021/acs.est.7b03040.

R. D. Braatz, M. Fujiwara, D. L. Ma, T. Togkalidou, and D. K. Tafti, “Simulation and new sensor technologies for industrial crystallization: A review,” Int. J. Mod. Phys. B, vol. 16, no. 1–2, pp. 346–353, 2002, doi: 10.1142/s0217979202009858.

L. Theodore and F. Ricci, Mass Transfer Operations for the Practicing Engineer. John Wiley & Sons, Inc., 2010.

C. J. Geankoplis, Transport processes and unit operations, Third edit., vol. 20, no. 1. Prentice-Hall International, Inc., 1993.

B. S. Choi, "Crystallization of sodium chloride from a concentrated calcium chloride-potassium chloride-sodium chloride solution in a CMSMPR crystallizer: Observation of crystal size distribution and model validation." PhD diss., The University of Utah, 2005.

W. L. McCabe, J. C. Smith, and P. Harriott, Unit Operation of Chemical Engineering, Fifth edit. McGraw-Hill, Inc., 1993.

J. Shanti and S. R. Vijayalakshmi, “Microcontroller Based Rotary Evaporator for Solution Growth,” Asian J. Adv. Basic Sci., vol. 3, no. 1, pp. 89–93, 2014.

S. Y. Misyura, “Different modes of heat transfer and crystallization in a drop of NaCl solution: The influence of key factors on the crystallization rate and the heat transfer coefficient,” Int. J. Therm. Sci., vol. 159, p. 106602, 2021, [Online].

A. Panagopoulos, K. J. Haralambous, and M. Loizidou, “Desalination brine disposal methods and treatment technologies - A review,” Sci. Total Environ., vol. 693, p. 133545, 2019, doi: 10.1016/j.scitotenv.2019.07.351.

E. T. Igunnu and G. Z. Chen, “Produced Water Treatment technologies,” Int. J. Low-Carbon Technol., vol. 9, pp. 157–177, 2014, doi: 10.2118/27177-ms.

M. H. Salih, A. F. Al-Alawy, and T. A. Ahmed, “Oil Skimming Followed by Coagulation/Flocculation Processes for Oilfield Produced Water Treatment and Zero Liquid Discharge System Application,” AIP Conf. Proc., vol. 2372, pp. 1–11, 2021. https://doi.org/10.1063/5.0065365

M. H. Salih and A. F. Al-alawy, “A novel forward osmosis for treatment of high-salinity East Baghdad oilfield produced water as a part of a zero liquid discharge system,” Desalin. Water Treat., vol. 248, pp. 18–27, 2022, doi: 10.5004/dwt.2022.28070. http://doi.org/10.5004/dwt.2022.28070

X. Chen, Q. Zheng, and Y. Dong, “Theoretical estimation of evaporation heat in paper drying process based on drying curve,” Processes, vol. 9, no. 7, pp. 1–11, 2021, doi: 10.3390/pr9071117.

A. F. Al-Alawy, “Forward and Reverse Osmosis Process for Recovery and Re-use of Water from Polluted Water by Phenol,” J. Eng., vol. 17, no. 4, pp. 912–928, 2011.

A. Naillon, P. Duru, M. Marcoux, and M. Prat, “Evaporation with sodium chloride crystallization in a capillary tube,” J. Cryst. Growth, vol. 422, pp. 52–61, 2015, doi: 10.1016/j.jcrysgro.2015.04.010.

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Published

2022-03-30

How to Cite

Salih, M. H., & Al-Alawy, A. F. (2022). Crystallization Process as a Final Part of Zero Liquid Discharge System for Treatment of East Baghdad Oilfield Produced Water. Iraqi Journal of Chemical and Petroleum Engineering, 23(1), 15-22. https://doi.org/10.31699/IJCPE.2022.1.3

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